From the games that I've played:
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Chrono Cross, there isn't much anything else like it
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Hotline Miami. Bastion. Portal 2. World of Warcraft, or W3, Dustforce... Probably many PS1, PS2, Gameboy, Gamecube, Sega games too but too many to remember.
The one I've heard the most is probably Bastion, tho. Those songs don't really feel like listening to game OSTs. They're just nice songs on their own right.
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Mass Effect and Final Fantasy X are great. My favorite is probably Mirrors Edge though.
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Battlefield 2: Modern Combat
https://www.youtube.com/watch?v=bxQObFA93V0&list=PLAC506814EB4AC831
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Man... That's one great OST. Never heard it before.
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The Witcher Series, Payday 1 + 2, Hitman Blood money :D
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So I made a movie soundtrack thread. Figured I'd make one for games. I'm gonna with the Elder Scrolls III: Morrowind
The main theme. The ingame music is great too though.
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