Homeworld, doesnt get better than that
Mass Effect 3
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Freelancer, XIII, Final Fantasy VIII (but this one is pretty much confirmed), Silent Hill 2, MGS 2, The Suffering and The Suffering 2
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First party Nintendo games will probably never happen. I don't mind playing them on the original console, though. Just better than a keyboard or a rekeyed controller to me, for some reason.
For anyone who (like myself) wonders why MC isn't on Steam... http://notch.tumblr.com/post/9550850116/why-no-steam-notch
(Hopefully they will eventually come to an agreement!)
Blizzard seems to be missing from the Steam scene. I suspect they will attempt to do the same thing that EA has and try to do their own gaming client. (Get with it, people! I really don't want a separate client for each publisher! Don't you see the potential profit you'd make just sticking with what's already the most popular?)
Shame, though: Diablo 2 would be an amazing addition to Steam, and I think it would introduce (and reintroduce) a new community of players to what is currently a predominantly bot-run and nearly desolate remnant of its former glory. Not gonna jump on the bandwagon of hate for D3, the game really is OK, but I played D2 for years and I can really see myself getting back into it if there was a resurgence in the community to keep it alive.
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Several that are on GOG only so far (Sanitarium being the prime example).
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I was just thinking about how that crappy "Castlevania" game came to Steam recently. I would absolutely buy the good ones in the franchise. Simon's Quest (maybe), Symphony of the Night, Aria of Sorrow, Harmony of Dissonance, and Dawn of Sorrow (use the mouse to draw the stupid symbols). Maybe even Circle of the Moon.
Since first-party Nintendo games including Super Metroid are out, Shadow Complex. It was a spiritual successor to Super Metroid released exclusively on Xbox Live Arcade a few years ago. The story was written by Orson Scott Card however, and a lot of people don't want their money going to hate groups, so that might be a problem. I might still buy it. Bought it on the 360 already, though.
If Square ever put Secret of Mana or Chrono Trigger on Steam I would definitely buy Mana, and probably pick up Chrono at some point.
So many anime games are exclusive to Sony. (Anybody know why that is?) The .hack//SIGN game, all four parts in one package (the game was divided into four parts for some reason). The Fullmetal Alchemist stuff.
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