Probably Braid, though I just finished Thomas Was Alone from the current humble bundle and I really loved that game.
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Saints Row: The Third from the Humble THQ Bundle =P
If we're not counting that bundle then probably Super Hexagon from the Humble Android Bundle 5
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Hard to say, so many choices to pick from, maybe Sol Survivor, Waking Mars, or Botanicula, I've gotten so many bundles though it's hard to keep track of what I've bought in a bundle :P
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So many to choose from, but Blackwell Deception is up there very high and the Groupees Wadjet Eye bundle was filled with some gems.
Also Legend of Grimrock, Saints Row 3, Machinarium, Amnesia, Anodyne.
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My favorite would be Bastion overall, especially as it included the soundtrack. From the current bundle I like Capsized.
Edit: I also had a good time in Dungeon Defenders, although I got it before it was bundled.
Edit2: Metro2033 was also good.
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